Combining Electrons and Lasers to Create Designer Beams for Materials Research

Tabletop laser systems generate extreme ultraviolet probes will advance research towards a new generation of energy-conserving electronics.

This artistically enhanced depiction shows an atom being hit by a strong rosette-shaped laser field (purple), ripping an electron (green) from the parent atom that then re-collides with the atom. — Image courtesy of Kapteyn/Murnane Group and Steve Burrows, Joint Institute for Laboratory Astrophysics and the Cohen Group, Technion University

The Science

Scientists developed a new probe to measure dynamic behavior of materials on ultrafast timescales. The extreme ultraviolet (EUV) probe is highly controlled (with respect to polarization, energy spectrum, and pulse shape) and can be used to extract dynamic information on electronic and magnetic properties. Lasers from tabletop systems create these probes by interacting with electrons in parent gas atoms, emitting EUV light.

The Impact

Tabletop-created designer beams of EUV and soft x-rays enable ultrafast spectroscopy measurements that are sensitive to the magnetic and electronic structure of materials. Ultrafast dynamics of energy flow (on the timescales of electron transitions and atomic lattice vibrations) are critical to understanding and discovering materials for energy-conserving next-generation electronics and information storage.

Summary

After a material is excited, the first electronic motions are fundamental processes that enable transport of energy and information. Snapshots of these ultrafast motions will further our understanding of the electronic structure of materials. However, probing the dynamics of electronic transitions and atomic-level energy flow requires using techniques with ultrafast time resolution. Here ultrafast is defined as the timescale of an electron transition or a single atomic vibration. Ultrafast responses can be probed with specialty pulsed beams. The beams can both excite the system and probe it stroboscopically. Such ultrafast “pump and probe” experiments require light that ranges into the EUV and soft x-ray regime, with unique spectral shape and polarization (that is, the direction of electromagnetic forces that the light creates in relation to the direction of the beam). High-power lasers from tabletop systems have been employed to create designer beams. The key to the technique is to match the sequence of crests in the wave of the laser beam with the wave of the outgoing designer beam, as they both travel through a gas. Two groups have recently been successful in doing just that: (1) One group created a pulsed beam with circular polarization that can detect the orientation of magnetic spins in a material through polarization dependent x-ray absorption. (2) The other created sharp pulses of energetic photons at a high repetition rate. These pulses can be used to measure photo-emitted electrons in small, repeated bunches before the electrons spread apart due to electrostatic repulsion. These new probes reveal information about the electronic structure in a material, such as the energy of electrons versus the momentum and direction travelled in a solid. The new probe sources will enable important studies of materials on the timescale of the electronic motion (both magnetic and charge) after an excitation—the fundamental processes that enable energy and information transport in solids.

Contact

Margaret Murnane
Joint Institute for Laboratory Astrophysics (JILA),
University of Colorado
[email protected]

Robert Kaindl
Lawrence Berkeley National Laboratory
[email protected]

Funding

This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; USA–Israel Binational Science Foundation, Israeli Centers for Research Excellence Program of the Planning and Budgeting Committee, and the Israel Science Foundation; the German Academic Exchange Service; the Deutsche Forschungsgemeinschaft; the Swedish Research Council; Air Force Office of Scientific Research-Defense University Research Instrumentation Program (laser system), and the National Science Foundation.

Publications

O. Kfir, P. Grychtol, E. Turgut, R. Knut D. Zusin, D. Popmintchev, T. Popmintchev, H. Nembach, J. Shaw, A. Fleicher, H. Kapteyn, M. Murnane, and O. Cohen, “Generation of bright circularly-polarized extreme ultraviolet high harmonics for magnetic circular dichroism spectroscopy.” Nature Photonics 9, 99 (2015). [DOI: 10.1038/nphoton.2014.293].

H. Wang, Y. Xu, S. Ulonska, J. S. Robinson, P. Ranitovic, and R. A. Kaindl, “Bright high-repetition-rate source of narrowband extreme-ultraviolet harmonics beyond 22 eV.” Nature Communications 6, 7459 (2015). [DOI: 10.1038/ncomms8459].