Magnetic Discovery Could Be Tip of the “Ice”berg

A material with unprecedented control of magnetic states may have implications for new technologies.

Image courtesy of Yong-Lei Wang, Zhi-Li Xiao, and Wai-Kwong Kwok, Argonne National Laboratory, University of Notre Dame, and Northern Illinois University.

The Science

A new material, called "rewritable magnetic charge ice," has an unprecedented degree of control over local magnetic fields. The artificial, magnetically charged structure is formed by manipulating local magnetic charges that set the state of the magnetic “bits.” This new magnetic charge-ice structure demonstrates write-read-erase capabilities at room temperature, which may have implications for new computing technologies.

The Impact

Scientists consider artificial spin ices to be scientific playgrounds, where the mysteries of magnetism might be explored and revealed. By using a new design method, the team tailored the artificial ice states in such a way that may enable their application for room temperature, rewritable data storage, memory, and logic devices, or in magnonics to study spin waves in nanostructures. Rather than focusing on spins, tackling the magnetic charges allows more controllability

Summary

Current magnetic storage and recording devices, such as computer hard disks, contain nanomagnets with two polarities, each of which is used to represent either 0 or 1 — the binary digits, or bits, used in computers. Over the past decade, scientists have been keenly interested in creating, investigating, and attempting to manipulate the unusual properties of "artificial spin ices." The materials are so named because the spins have a lattice structure that follows the proton positioning ordering found in water ice. A magnetic charge ice system could have eight possible configurations instead of two, resulting in denser storage capabilities or added functionality unavailable in current technologies. However, in the past, researchers have been frustrated in their attempts to achieve global and local control of spin-ice magnetic charges. To overcome this challenge, a research team from Argonne National Laboratory, including the Center for Nanoscale Materials (CNM), University of Notre Dame, and Northern Illinois University decoupled the lattice structure of magnetic spins and the magnetic charges. Decoupling the structure and the charges allowed them to precisely and conveniently tune the magnetic charge ice to any of eight possible charge configurations. The configurations are two in a Type I ground state, two in a Type II (two-fold symmetric) excited state, and four in a Type III (four-fold symmetric) excited state. The team used electron beam lithography at CNM to pattern the samples, and a magnetic force microscope equipped with a two-dimensional vector magnet (capable of fine tuning the applied field strength and direction) to demonstrate the array’s local write-read-erase multi-functionality at room temperature.

Contact

Wai-Kwong Kwok ([email protected]), Materials Science Division, Argonne National Laboratory

Yong-Lei Wang ([email protected]), University of Notre Dame and Argonne National Laboratory

Zhi-Li Xiao ([email protected]), Northern Illinois University and Argonne National Laboratory

Leonidas E. Ocola ([email protected]) and Ralu Divan ([email protected]), Center for Nanoscale Materials
Argonne National Laboratory

Funding

This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, including use of the Center for Nanoscale Materials, an Office of Science user facility. Z.L.X. and J.X. were supported by the National Science Foundation.

Publications

Y. L. Wang, Z.L. Xiao, A. Snezhko, J. Xu, L.E. Ocola, R. Divan, J.E. Pearson, G.W. Crabtree, and W.K. Kwok, “Rewritable artificial magnetic charge ice.” Science 352, 962 (2016). [DOI: 10.1126/science.aad8037]